On flow masers with separated emission fields

Abstract

In 1954 the invention of the ammonia molecular beam maser oscillator, through Charles Hard TOWNES and co-workers and Nikolai Gennadievich BASOV and Alexander Mikhailovich PROKHOROV, opened a new area of applied physics, the field of quantum electronics. Ten years later the importance of the invention of the new device which consists essentially of a microwave resonator and excited ammonia molecules which pass through the resonator was acknowledged by the award of the 1964 NOBEL Prize in physics to the above workers.
Soon after the invention of the maser principle, an ammonia beam maser utilizing separated emission fields was brought into operation, a device which consists of two separated microwave resonators through which the ammonia beam maser passes in succession. It is now well known that this two-cavity variant has great practical advantages over the original one-cavity ammonia beam maser.
However, not all of the macroscopic effects observed using the two-cavity ammonia beam maser could be explained in a straight­forward manner. One of the more obscure effects presents itself as follows: If the frequency of the auto-oscillation in the first resonator is detuned from one side of the possible frequency range in which generation occurs to the other then the intensity of the electromagnetic radiation in the second cavity can go through two maxima, with a gap in the middle.
This effect, the "double-hump detuning phenomenon", which was first observed by the Russian research group of BASOV in 1962, has since then been a challenge to several theoretical and experimental workers. BASOV and co-workers themselves made two different attempts in order to explain this phenomenon. At the Third International Conference on Quantum Electronics, held in Paris in 1963, this team reported that the effect might occur because the transition probability of the molecules passing through the second resonator depends on the degree of excitation of the first cavity. However, in 1967 BASOV and co-workers published a paper where it is suggested that the double-hump detuning phenomenon might well arise because of the interference which occurs between the emissions from molecules which move with different velocities and radiate fields with different phases.
On the other hand, research activities in fields other than microwave spectroscopy have made it possible to devise masers which are similar to the ammonia beam maser in that excited particles pass through a tuned resonant component, but which emit at quite different frequencies, e.g. in the audio-frequency ranee or in the mm wave range. However, up to now none of these different masers has been furnished with a successive resonator.
It is the purpose of this thesis to report for the first time the successful operation of a tandem maser which is not a two-cavity molecular beam maser. The author devised and investigated a maser where excited protons in water pass successively through two tuned solenoids.
The system is based on a conventional proton magnetometer maser oscillating in the magnetic field of the earth at a frequency near to 2 kHz.
The general result of the investigation is that despite
the enormous frequency difference (audio-frequency compared with a microwave frequency) the two coil nuclear maser behaves in much the same way as a two cavity ammonia beam maser. For the two-coil nuclear maser the double-hump detuning phenomenon can be explained
in terms of the motion of the macroscopic nuclear magnetization, and an analysis by means of BLOCH'S equations is possible. It is shown that the double-hump detuning phenomenon is produced by a fundamental radiation process occurring in the first emission coil and 1 therefore, that it is not a second-order effect such as could occur because of the non-uniform velocity distribution of the excited particles.
It is also shown that for the two-resonator ammonia beam maser the detuning phenomenon can be explained in terms of quantum mechanical probabilities, when a uniform velocity distribution of the ammonia molecules is assumed. Those results agree qualitatively with the results which have been obtained using BLOCH's equations and which have been verified experimentally by means of the two-coil nuclear maser.
A second distinctive feature of the conventional two-cavity ammonia beam maser is that if the first resonator is sufficiently detuned, generation in the second resonator can take place simultaneously at two different frequencies. The analogous effect has been observed using the two-coil nuclear maser.
The conventional one-coil nuclear maser which is currently used as a magnetometer has the disadvantage that it does not offer a suitable criterion for tuning the oscillation frequency accurately to the LARMOR frequency. For the two-cavity ammonia beam maser it has previously been proposed to modulate mechanically the inter-cavity distance and to use zero phase modulation as a means of tuning the maser frequency accurately to the centre frequency of the molecular transition. It is shown that by modulating mechanically the inter­coil distance of the two-coil nuclear maser. a suitable tuning criterion can be obtained in an analogous manner. A second tuning criterion is offered by the double-hump detuning phenomenon.
In Chapter I the maser principle is discussed using a classical model, and the different maser types which are of interest in the context of this thesis are enumerated. Chapter II contains a review of previous work on two-cavity ammonia beam masers.
Chapter III reviews the conventional theory of nuclear masers. In Chapters IV to IX the two-coil nuclear maser is investigated. Chapter X contains a general discussion of the two-resonator maser problem in terms of quantum-mechanical probabilities. Some general remarks concerning practical applications of two-resonator masers
are made. The conclusions are summarized in a final section.